Source code for openqemist.quantum_solvers.microsoft_qsharp.integrals_pyscf

#   Copyright 2019 1QBit
#   
#   Licensed under the Apache License, Version 2.0 (the "License");
#   you may not use this file except in compliance with the License.
#   You may obtain a copy of the License at
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#       http://www.apache.org/licenses/LICENSE-2.0
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#   Unless required by applicable law or agreed to in writing, software
#   distributed under the License is distributed on an "AS IS" BASIS,
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#   See the License for the specific language governing permissions and
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import numpy as np

[docs]def compute_integrals_fragment(mol, myhf): """ Compute the electronic integrals and store them in a data-structure that can be used by MicrosoftQSharp backend """ from pyscf import gto, scf, fci, ao2mo n_orbitals = len(myhf.mo_energy) # One electron integrals: compute with PySCF, then thresholds and prepare for Microsoft data-structure one_electron_compressed = myhf.mo_coeff.T @ myhf.get_hcore() @ myhf.mo_coeff t1 = one_electron_compressed.reshape(n_orbitals, n_orbitals).astype(float) t1_thresh = np.around(t1, decimals=6) t1_bb = [([int(j+1), int(i+1)], t1_thresh[i, j]) for i in range(t1_thresh.shape[0]) for j in range(i, t1_thresh.shape[1]) if t1_thresh[i, j] != 0.] # Two electron integrals: compute with PySCF, then thresholds and prepare for Microsoft data-structure # The following occasionally returned a PySCF bug. It was replaced by the snippet below #two_electron_compressed = ao2mo.kernel(mol, myhf.mo_coeff) #t2 = ao2mo.restore(1, two_electron_compressed, n_orbitals) twoint=myhf._eri eri= ao2mo.restore(8,twoint,n_orbitals) eri= ao2mo.incore.full(eri,myhf.mo_coeff) t2 = ao2mo.restore(1,eri,n_orbitals) # Store entries for non-zero integrals only if they are not a permutation # of an existing entry def is_two_body_permutation(coords1, coords2): """ Test if coords are two-electorn permutations in mulliken convention """ return ( coords1 == [coords2[i] for i in [0, 1, 2, 3]] or coords1 == [coords2[i] for i in [2, 3, 0, 1]] or coords1 == [coords2[i] for i in [1, 0, 3, 2]] or coords1 == [coords2[i] for i in [3, 2, 1, 0]] or coords1 == [coords2[i] for i in [1, 0, 2, 3]] or coords1 == [coords2[i] for i in [3, 2, 0, 1]] or coords1 == [coords2[i] for i in [0, 1, 3, 2]] or coords1 == [coords2[i] for i in [2, 3, 1, 0]]) t2_thresh = np.around(t2, decimals=6) values, indices = [], [] for (coords, value) in np.ndenumerate(t2_thresh): if value == 0.: continue else : coords = list(coords) new_integral = True for coords_ref in indices: if is_two_body_permutation(coords_ref, coords): new_integral = False if new_integral: values.append(value) indices.append(coords) # Convert two-electron integrals to Broombridge format t2_bb = [[int(coord+1) for coord in coords] for coords in indices] t2_bb = [(t2_bb[i], values[i]) for i in range(len(t2_bb))] return t1_bb, t2_bb